It's better to work in 1-forms to see what's going on. We can think of a one-form λ as a section s:X→T∗X by pulling back the Liouville form s∗θ=λ. The symplectic form is dθ so the "curl" from this roundabout construction is s∗dθ=ds∗θ=dλ, so curl is just dual (in the sense that 1-forms correspond to vector fields by line integrals) to the exterior derivative, which is ubiquitous in geometry and physics.
Here is a geometric interpretation of the curl: it's a 2-form, so it takes a value on each tangent plane. If one projects the vector field onto this plane and computes the usual 2d curl it will be the value of the 2-form curl on this tangent plane.